Hello @杉山 明宏
Thank you for reaching out to the Microsoft Q&A forum.
Based on the information you shared, I understand that you are experiencing an issue where Outlook on your iPhone is not syncing sent and received emails correctly. You mentioned that this issue first occurred when your mailbox reached its maximum storage limit, and even after extending the storage, the problem has not yet been resolved.
To help refresh the connection and resync your mailbox, please try resetting your account in the Outlook app on your iPhone by following the steps below:
- Open the Outlook app on your iPhone.
- Tap Settings.
- Scroll down and, under the General section, select Accounts.
- Choose the account that is experiencing the issue.
- Scroll to the bottom and tap Reset Account.
After completing these steps, please allow a few minutes for the mailbox to resync. Then, check whether your emails are now sending, receiving, and syncing correctly.
Kindly let me know the outcome after trying the steps above, and I will be happy to assist you further if needed. I look forward to hearing from you.